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Aviation 2006 NoX-induced Effects on Atmospheric Ozone and HoX in Community Earth System Model (Cesm) : Volume 14, Issue 18 (19/09/2014)

By Khodayari, A.

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Book Id: WPLBN0003989995
Format Type: PDF Article :
File Size: Pages 15
Reproduction Date: 2015

Title: Aviation 2006 NoX-induced Effects on Atmospheric Ozone and HoX in Community Earth System Model (Cesm) : Volume 14, Issue 18 (19/09/2014)  
Author: Khodayari, A.
Volume: Vol. 14, Issue 18
Language: English
Subject: Science, Atmospheric, Chemistry
Collections: Periodicals: Journal and Magazine Collection (Contemporary), Copernicus GmbH
Publication Date:
Publisher: Copernicus Gmbh, Göttingen, Germany
Member Page: Copernicus Publications


APA MLA Chicago

Lamarque, J., Tilmes, S., Khodayari, A., Chen, C., Phoenix, D. B., Olsen, S. C., & Wuebbles, D. J. (2014). Aviation 2006 NoX-induced Effects on Atmospheric Ozone and HoX in Community Earth System Model (Cesm) : Volume 14, Issue 18 (19/09/2014). Retrieved from

Description: Department of Civil and Environmental Engineering, University of Illinois at Urbana-Champaign, Urbana, IL 61801, USA. The interaction between atmospheric chemistry and ozone (O3) in the upper troposphere–lower stratosphere (UTLS) presents a major uncertainty in understanding the effects of aviation on climate. In this study, two configurations of the atmospheric model from the Community Earth System Model (CESM), Community Atmosphere Model with Chemistry, Version 4 (CAM4) and Version 5 (CAM5), are used to evaluate the effects of aircraft nitrogen oxide (NOx = NO + NO2) emissions on ozone and the background chemistry in the UTLS. CAM4 and CAM5 simulations were both performed with extensive tropospheric and stratospheric chemistry including 133 species and 330 photochemical reactions. CAM5 includes direct and indirect aerosol effects on clouds using a modal aerosol module (MAM), whereby CAM4 uses a bulk aerosol module, which can only simulate the direct effect. To examine the accuracy of the aviation NOx-induced ozone distribution in the two models, results from the CAM5 and CAM4 simulations are compared to ozonesonde data. Aviation NOx emissions for 2006 were obtained from the AEDT (Aviation Environmental Design Tool) global commercial aircraft emissions inventory. Differences between simulated O3 concentrations and ozonesonde measurements averaged at representative levels in the troposphere and different regions are 13% in CAM5 and 18% in CAM4. Results show a localized increase in aviation-induced O3 concentrations at aviation cruise altitudes that stretches from 40° N to the North Pole. The results indicate a greater and more disperse production of aviation NOx-induced ozone in CAM5, with the annual tropospheric mean O3 perturbation of 1.2 ppb (2.4%) for CAM5 and 1.0 ppb (1.9%) for CAM4. The annual mean O3 perturbation peaks at about 8.2 ppb (6.4%) and 8.8 ppb (5.2%) in CAM5 and CAM4, respectively. Aviation emissions also result in increased hydroxyl radical (OH) concentrations and methane (CH4) loss rates, reducing the tropospheric methane lifetime in CAM5 and CAM4 by 1.69 and 1.40%, respectively. Aviation NOx emissions are associated with an instantaneous change in global mean short-term O3 radiative forcing (RF) of 40.3 and 36.5 mWm−2 in CAM5 and CAM4, respectively.

Aviation 2006 NOx-induced effects on atmospheric ozone and HOx in Community Earth System Model (CESM)

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